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121.
Neal T. Skipper Peter A. Lock James O. Titiloye Jan Swenson Zakaria A. Mirza W. Spencer Howells Felix Fernandez-Alonso 《Chemical Geology》2006,230(3-4):182-196
The interlayer pores of swelling 2:1 clays provide an ideal 2-dimensional environment in which to study confined fluids. In this paper we discuss our understanding of the structure and dynamics of interlayer fluid species in expanded clays, based primarily on the outcome of recent molecular modelling and neutron scattering studies. Counterion solvation is compared with that measured in bulk solutions, and at a local level the cation-oxygen coordination is found to be remarkably similar in these two environments. However, for the monovalent ions the contribution to the first coordination shell from the clay surfaces increases with counterion radius. This gives rise to inner-sphere (surface) complexes in the case of potassium and caesium. In this context, the location of the negative clay surface charge (i.e. arising from octahedral or tetrahedral substitution) is also found to be of major importance. Divalent cations, such as calcium, eagerly solvate to form outer-sphere complexes. These complexes are able to pin adjacent clay layers together, and thereby prevent colloidal swelling. Confined water molecules form hydrogen bonds to each other and to the clays' surfaces. In this way their local environment relaxes to close to the bulk water structure within two molecular layers of the clay surface. Finally, we discuss the way in which the simple organic molecules methane, methanol and ethylene glycol behave in the interlayer region of hydrated clays. Quasi-elastic neutron scattering of isotopically labelled interlayer CH3OD and (CH2OD)2 in deuterated clay allows us to measure the diffusion of the CH3- and CH2-groups in both clay and liquid environments. We find that in both the one-layer methanol solvates and the two-layer glycol solvates the diffusion of the most mobile organic molecules is close to that in the bulk solution. 相似文献
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123.
Thomas A. Vogel Timothy P. Flood Lina C. Patino Melissa S. Wilmot Raymond Patrick R. Maximo Carmencita B. Arpa Carlo A. Arcilla James A. Stimac 《Contributions to Mineralogy and Petrology》2006,151(3):267-281
Silicic volcanic deposits (>65 wt% SiO2), which occur as domes, lavas and pyroclastic deposits, are relatively abundant in the Macolod Corridor, SW Luzon, Philippines.
At Makiling stratovolcano, silicic domes occur along the margins of the volcano and are chemically similar to the silicic
lavas that comprise part of the volcano. Pyroclastic flows are associated with the Laguna de Bay Caldera and these are chemically
distinct from the domes and lavas at Makiling stratovolcano. As a whole, samples from the Laguna de Bay Caldera contain lower
concentrations of MgO and higher concentrations of Fe2O3(t) than the samples from domes and lavas. The Laguna de Bay samples are more enriched in incompatible trace elements. The silicic
rocks from the domes, Makiling Volcano and Laguna de Bay Caldera all contain high alkalis and high K2O/Na2O ratios. Melting experiments of primitive basalts and andesites demonstrate that it is difficult to produce high K2O/Na2O silicic magmas by fractional crystallization or partial melting of a low K2O/Na2O source. However, recent melting experiments (Sisson et al., Contrib Mineral Petrol 148:635–661, 2005) demonstrate that extreme
fractional crystallization or partial melting of K-rich basalts can produce these silicic magmas. Our model for the generation
of the silicic magmas in the Macolod Corridor requires partial melting of mantle-derived, evolved, moderate to K-rich, crystallized
calc-alkaline magmas that ponded and crystallized in the mid-crust. Major and trace element variations, along with oxygen
isotopes and ages of the deposits, are consistent with this model.
Electronic Supplementary Material Supplementary material is available for this article at 相似文献
124.
James L. Crowley Mark D. Schmitz Samuel A. Bowring Michael L. Williams Karl E. Karlstrom 《Contributions to Mineralogy and Petrology》2006,151(3):313-330
Zircon from lower crustal xenoliths erupted in the Navajo volcanic field was analyzed for U–Pb and Lu–Hf isotopic compositions
to characterize the lower crust beneath the Colorado Plateau and to determine whether it was affected by ∼1.4 Ga granitic
magmatism and metamorphism that profoundly affected the exposed middle crust of southwestern Laurentia. Igneous zircon in
felsic xenoliths crystallized at 1.73 and 1.65 Ga, and igneous zircon in mafic xenoliths crystallized at 1.43 Ga. Most igneous
zircon has unradiogenic initial Hf isotopic compositions (ɛHf=+4.1–+7.8) and 1.7–1.6 Ga depleted mantle model ages, consistent with 1.7–1.6 Ga felsic protoliths being derived from “juvenile”
Proterozoic crust and 1.4 Ga mafic protoliths having interacted with older crust. Metamorphic zircon grew in four pulses between
1.42 and 1.36 Ga, at least one of which was at granulite facies. Significant variability within and between xenoliths in
metamorphic zircon initial Hf isotopic compositions (ɛHf=−0.7 to +13.6) indicates growth from different aged sources with diverse time-integrated Lu/Hf ratios. These results show
a strong link between 1.4 Ga mafic magmatism and granulite facies metamorphism in the lower crust and granitic magmatism and
metamorphism in the exposed middle crust. 相似文献
125.
Racism has become a fact of life in Australia over the past decade or so, yet there are relatively few studies of its nature or extent, and still fewer on its geography. Using a social constructivist approach, this study draws on a survey of 5056 respondents to investigate attitudes to racism and cultural diversity in New South Wales and Queensland, and of perceptions of out-groups as instances of ‘strangers in our midst’. On racism, results show the presence of a continuum of attitudes ranging from generally tolerant to generally intolerant, a presence which cuts across compositional (social or aspatial) characteristics to emphasise the existence of a distinctive geography, an everywhere different nature to racist and non-racist attitudes which transcends urban–rural and traditional social layers. On the other hand, perceptions of out-groups are not uniformly correlated with presence or absence of cultural diversity. In many cases, the ability to make judgements about significant ‘others’ or out-groups has been shown to relate more to abstract notions of self and national identity, reproduced in public by mainstream news media and political leaders. In particular, it may reflect an Anglo (or Anglo-Celtic) view on nationalism, which is a hallmark of the ‘new racism’: an assimilationist or ethnocultural view of Australian society which is different from the ‘civic nation’ ideal envisaged by multiculturalism. That the geography of attitudes and perceptions people have towards and about different cultural groups is so ‘everywhere different’ has important implications for attempts to address and redress issues of intolerance in Australia. 相似文献
126.
127.
128.
Brian Emmerson James Jackson Dan McKenzie Keith Priestley 《Geophysical Journal International》2006,167(3):1233-1272
129.
Trevor Quinn A.-Xing Zhu James E. Burt 《International Journal of Applied Earth Observation and Geoinformation》2005,7(4):324-338
Hydro-ecological modelers often use spatial variation of soil information derived from conventional soil surveys in simulation of hydro-ecological processes over watersheds at mesoscale (10–100 km2). Conventional soil surveys are not designed to provide the same level of spatial detail as terrain and vegetation inputs derived from digital terrain analysis and remote sensing techniques. Soil property layers derived from conventional soil surveys are often incompatible with detailed terrain and remotely sensed data due to their difference in scales. The objective of this research is to examine the effect of scale incompatibility between soil information and the detailed digital terrain data and remotely sensed information by comparing simulations of watershed processes based on the conventional soil map and those simulations based on detailed soil information across different simulation scales. The detailed soil spatial information was derived using a GIS (geographical information system), expert knowledge, and fuzzy logic based predictive mapping approach (Soil Land Inference Model, SoLIM). The Regional Hydro-Ecological Simulation System (RHESSys) is used to simulate two watershed processes: net photosynthesis and stream flow. The difference between simulation based on the conventional soil map and that based on the detailed predictive soil map at a given simulation scale is perceived to be the effect of scale incompatibility between conventional soil data and the rest of the (more detailed) data layers at that scale. Two modeling approaches were taken in this study: the lumped parameter approach and the distributed parameter approach. The results over two small watersheds indicate that the effect does not necessarily always increase or decrease as the simulation scale becomes finer or coarser. For a given watershed there seems to be a fixed scale at which the effect is consistently low for the simulated processes with both the lumped parameter approach and the distributed parameter approach. 相似文献
130.